Synthetic peptides caged on histidine residues with a bisbipyridyl ruthenium(II) complex that can be photolyzed by visible light

We report a light-sensitive histidine building block for Fmoc/tBu solid-phase peptide synthesis in which the imidazole side chain is coordinated to a ruthenium complex. We have applied this building block for the synthesis of caged-histidine peptides that can be readily deprotected by irradiation wi...

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Detalhes bibliográficos
Autores: Mosquera Mosquera, Jesús, Sánchez López, Mateo Isidro, Mascareñas Cid, José Luis, Vázquez Sentís, Marco Eugenio
Formato: artículo
Fecha de publicación:2015
País:España
Recursos:Universidad de Santiago de Compostela (USC)
Repositorio:Minerva. Repositorio Institucional de la Universidad de Santiago de Compostela
Idioma:inglés
OAI Identifier:oai:minerva.usc.gal:10347/12547
Acesso em linha:http://hdl.handle.net/10347/12547
Access Level:acceso abierto
Palavra-chave:Materias::Investigación::23 Química::2302 Bioquímica
Descrição
Resumo:We report a light-sensitive histidine building block for Fmoc/tBu solid-phase peptide synthesis in which the imidazole side chain is coordinated to a ruthenium complex. We have applied this building block for the synthesis of caged-histidine peptides that can be readily deprotected by irradiation with visible light, and demonstrated the application of this approach for the photocontrol of the activity of Ni(II)-dependent peptide nucleases