Fractional statistical theory of finite multilayer adsorption

In the present paper, finite multilayer adsorption is described as a fractional statistics problem, based on Haldane's statistics. In this scheme, the Helmholtz free energy and its derivatives are written in terms of a parameter g, which relates to the configuration of the molecules in the adso...

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Detalhes bibliográficos
Autores: Takara, Eduardo Andres, Quiroga, Evelina, Matoz Fernandez, Daniel Alejandro, Ochoa, Nelio Ariel, Ramirez Pastor, Antonio Jose
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2016
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositório:CONICET Digital (CONICET)
Idioma:inglês
OAI Identifier:oai:ri.conicet.gov.ar:11336/60469
Acesso em linha:http://hdl.handle.net/11336/60469
Access Level:Acceso aberto
Palavra-chave:Adsorption Isotherms
Bsa Protein Adsorption
Equilibrium Thermodynamics And Statistical Mechanics
Multilayer Adsorption
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descrição
Resumo:In the present paper, finite multilayer adsorption is described as a fractional statistics problem, based on Haldane's statistics. In this scheme, the Helmholtz free energy and its derivatives are written in terms of a parameter g, which relates to the configuration of the molecules in the adsorbed state. For values of g ranging between 0 and 1 the formalism is used to model experimental data of bovine serum albumin (BSA) adsorbed onto an ion exchange resin for different values of pH and temperature. Excellent agreement between theory and experiments was found.