Magnetoelastic coupling in La_(0.7)Ca_(0.3)MnO_(3)/BaTiO_(3) ultrathin films
The magnetism of La_(0.7)Ca_(0.3)MnO_(3) (LCMO) epitaxial thin films grown on SrTiO_(3) (STO) and BaTiO_(3) (BTO) substrates is studied using polarized neutron reflectometry (PNR) and ferromagnetic resonance (FMR) techniques. In LCMO/BTO, PNR reveals a strongly suppressed magnetization of 300 kA/m,...
| Autores: | , , , , , , , , , , , , |
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| Tipo de documento: | artigo |
| Data de publicação: | 2013 |
| País: | España |
| Recursos: | Universidad Complutense de Madrid (UCM) |
| Repositório: | Docta Complutense |
| Idioma: | inglês |
| OAI Identifier: | oai:docta.ucm.es:20.500.14352/34770 |
| Acesso em linha: | https://hdl.handle.net/20.500.14352/34770 |
| Access Level: | Acceso aberto |
| Palavra-chave: | 537 538.9 Magnetic-anisotropy Oxides. Electricidad Electrónica (Física) Física de materiales Física del estado sólido 2202.03 Electricidad 2211 Física del Estado Sólido |
| Resumo: | The magnetism of La_(0.7)Ca_(0.3)MnO_(3) (LCMO) epitaxial thin films grown on SrTiO_(3) (STO) and BaTiO_(3) (BTO) substrates is studied using polarized neutron reflectometry (PNR) and ferromagnetic resonance (FMR) techniques. In LCMO/BTO, PNR reveals a strongly suppressed magnetization of 300 kA/m, equivalent to a magnetic moment of 2 μB/Mn, throughout the LCMO layer, amounting to half the expected value. The largest suppression occurs near the interface with BTO, with magnetization values of 50 kA/m, equivalent to 0.3 μB/Mn. FMR is observable at 8.9 GHz only around the [110] crystallographic direction in thin LCMO/BTO. The resonance barely shifts as the applied field is rotated away from [110]. The FMR results are analyzed in terms of magnetoelastic anisotropy and compared to LCMO/STO grown under the same conditions. A two-layer magnetization model is proposed, based on strong out-of-plane anisotropy near the BTO interface and shown to qualitatively explain the main characteristics of the FMR results. |
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