Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets
4 pages, 4 figures.-- PACS nrs.: 36.40.–c, 33.20.Fb, 61.46.+w.
| Authors: | , , , , |
|---|---|
| Format: | article |
| Publication Date: | 2004 |
| Country: | España |
| Institution: | Consejo Superior de Investigaciones Científicas (CSIC) |
| Repository: | DIGITAL.CSIC. Repositorio Institucional del CSIC |
| OAI Identifier: | oai:digital.csic.es:10261/9014 |
| Online Access: | http://hdl.handle.net/10261/9014 |
| Access Level: | Open access |
| Keyword: | [PACS] Atomic and molecular clusters [PACS] Raman and Rayleigh spectra (including optical scattering) [PACS] Nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals |
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Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free JetsTejeda, GuzmánFernández Sánchez, José MaríaMontero, SalvadorBlume, D.Toennies, J.P.[PACS] Atomic and molecular clusters[PACS] Raman and Rayleigh spectra (including optical scattering)[PACS] Nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals4 pages, 4 figures.-- PACS nrs.: 36.40.–c, 33.20.Fb, 61.46.+w.Small para-H2 clusters (pH2)N with N=2,...,8 have been identified by Raman spectroscopy in cryogenic free jets of the pure gas, near the Q(0) Raman line of the H2 monomer. The high resolution in space, time, and number size makes it possible to follow their growth kinetics with distance from the orifice. At lower source temperatures liquid clusters appear early in the expansion and then undergo a gradual phase transition to the solid state. The technique is very promising for exploring superfluidity in pure (pH2)N clustersThis work was supported by the Spanish DGI (MCyT), research project No. BFM2001-2265. D. B. acknowledges support from the Petroleum Research Fund and the NSF.Peer reviewedAmerican Physical Society200820082004info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501325949 bytesapplication/pdfhttp://hdl.handle.net/10261/9014reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Ingléshttp://dx.doi.org/10.1103/PhysRevLett.92.223401info:eu-repo/semantics/openAccessoai:digital.csic.es:10261/90142026-05-22T06:33:51Z |
| dc.title.none.fl_str_mv |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| title |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| spellingShingle |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets Tejeda, Guzmán [PACS] Atomic and molecular clusters [PACS] Raman and Rayleigh spectra (including optical scattering) [PACS] Nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals |
| title_short |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| title_full |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| title_fullStr |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| title_full_unstemmed |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| title_sort |
Raman Spectroscopy of Small Para-H2 Clusters Formed in Cryogenic Free Jets |
| dc.creator.none.fl_str_mv |
Tejeda, Guzmán Fernández Sánchez, José María Montero, Salvador Blume, D. Toennies, J.P. |
| author |
Tejeda, Guzmán |
| author_facet |
Tejeda, Guzmán Fernández Sánchez, José María Montero, Salvador Blume, D. Toennies, J.P. |
| author_role |
author |
| author2 |
Fernández Sánchez, José María Montero, Salvador Blume, D. Toennies, J.P. |
| author2_role |
author author author author |
| dc.subject.none.fl_str_mv |
[PACS] Atomic and molecular clusters [PACS] Raman and Rayleigh spectra (including optical scattering) [PACS] Nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals |
| topic |
[PACS] Atomic and molecular clusters [PACS] Raman and Rayleigh spectra (including optical scattering) [PACS] Nanoscale materials: clusters, nanoparticles, nanotubes, and nanocrystals |
| description |
4 pages, 4 figures.-- PACS nrs.: 36.40.–c, 33.20.Fb, 61.46.+w. |
| publishDate |
2004 |
| dc.date.none.fl_str_mv |
2004 2008 2008 |
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info:eu-repo/semantics/article http://purl.org/coar/resource_type/c_6501 |
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article |
| dc.identifier.none.fl_str_mv |
http://hdl.handle.net/10261/9014 |
| url |
http://hdl.handle.net/10261/9014 |
| dc.language.none.fl_str_mv |
Inglés |
| language_invalid_str_mv |
Inglés |
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http://dx.doi.org/10.1103/PhysRevLett.92.223401 |
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info:eu-repo/semantics/openAccess |
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openAccess |
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325949 bytes application/pdf |
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American Physical Society |
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American Physical Society |
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