Microscale titration of acetic acid using digital colorimetry and paper-based analytical devices

A quantitative method for acid-base titrations in paper-based devices (PADs) is described to analyze acetic acid in vinegar samples. In this work, two different types of PADs were developed: a device for individual spot testing and a microfluidic device. Digital colorimetry was used as the detection...

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Detalhes bibliográficos
Autores: Berasarte Urroz, Irati, Bordagaray Eizaguirre, Ane, García Arrona, Rosa María, Ostra Beldarrain, Miren, Reis de Araujo, William, Vidal Postigo, Maider
Formato: artículo
Fecha de publicación:2024
País:España
Recursos:Universidad del País Vasco
Repositorio:Addi. Archivo Digital para la Docencia y la Investigación
OAI Identifier:oai:addi.ehu.eus:10810/69325
Acesso em linha:http://hdl.handle.net/10810/69325
Access Level:acceso abierto
Palavra-chave:paper-based device
micro-titration
paper microfluidics
colorimetry
digital image analysis
process automation
Descrição
Resumo:A quantitative method for acid-base titrations in paper-based devices (PADs) is described to analyze acetic acid in vinegar samples. In this work, two different types of PADs were developed: a device for individual spot testing and a microfluidic device. Digital colorimetry was used as the detection method, and the images were acquired using a smartphone and a homemade box with LED lights for controlled image acquisition. Titration curves were built with just eight points, using the R channel based on the gradual color transition from red to blue of litmus, a natural indicator. The endpoint was accurately determined by second derivative calculations. Both systems were applied to fifteen vinegar samples of different types, and good concentration results were obtained in comparison to the reference method. The proposed methodology is simple, fast, environmentally friendly, and surpasses the need for calibration curve construction. Moreover, the subjective endpoint identification is eliminated, and the method was automated to provide a high throughput workflow, suitable for quality control processes and real-time measurements.