Electrochemical study of tailored sol-gel thin films as pre-treatment prior to organic coating for AZ91 magnesium alloy

The behaviour/resistance of four optimised sol-gel coating systems (inorganic, hybrid organic-inorganic, containing zirconium ions and containing cerium ions) against corrosion of AZ91 magnesium alloy were studied. The coatings obtained by the sol-gel process were evaluated as autonomous protective...

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Detalhes bibliográficos
Autores: Barranco, Violeta, Carmona, N., Galván Sierra, Juan Carlos, Grobelny, M., Kwiatkowski, L., Villegas Broncano, María Ángeles
Tipo de documento: artigo
Estado:Versión enviada para evaluación y publicación
Data de publicação:2010
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositório:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/114611
Acesso em linha:http://hdl.handle.net/10261/114611
Access Level:Acceso aberto
Palavra-chave:Local electrochemical impedance spectroscopy (LEIS)
Electrochemical impedance spectroscopy (EIS)
Corrosion inhibitors
Cerium-doped coatings
Hybrid coatings
Sol–gel coatings
Descrição
Resumo:The behaviour/resistance of four optimised sol-gel coating systems (inorganic, hybrid organic-inorganic, containing zirconium ions and containing cerium ions) against corrosion of AZ91 magnesium alloy were studied. The coatings obtained by the sol-gel process were evaluated as autonomous protective coatings as well as a pre-treatment prior to acrylic top coat. The coating obtained from tetramethoxysilane (TMOS) and diethoxydimethylsilane (DEDMS) as precursors and doped with Ce3+ was especially effective as pre-treatment for a final acrylic coating. For non-defected coating the impedance modulus has not changed during the time of immersion (7 days) in 0.5 M Na2SO4. An inhibition of coating delamination at the defect of the acrylic coating was recorded by means of LEIS. © 2010 Elsevier B.V. All rights reserved.