Relating microhardness to morphology in styrene/butadiene block copolymer/polystyrene blends

The microhardness behaviour of binary blends comprising a styrene/butadiene star block copolymer and polystyrene homopolymer (hPS) over a wide composition range is investigated. In particular, the interrelation between the morphology, tensile properties (such as yield stress sY and the Young’s modul...

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Detalhes bibliográficos
Autores: Baltá Calleja, Francisco José, Cagiao, M. E., Adhikari, R., Michler, G.H.
Tipo de documento: artigo
Data de publicação:2004
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositório:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/79477
Acesso em linha:http://hdl.handle.net/10261/79477
Access Level:Acceso aberto
Palavra-chave:Styrene/butadiene block copolymer/polystyrene blends
Microhardness
Electron microscopy
Descrição
Resumo:The microhardness behaviour of binary blends comprising a styrene/butadiene star block copolymer and polystyrene homopolymer (hPS) over a wide composition range is investigated. In particular, the interrelation between the morphology, tensile properties (such as yield stress sY and the Young’s modulus, E) and the microhardness H is explored. As in the case of microphase separated block copolymers and binary block copolymer blends, as reported in preceding publications, a clear deviation in the microhardness behaviour from the additivity law is observed. The lamellar block copolymer system is compared with the nanostructure of semicrystalline polymers having a lamellar morphology. A dependence of H upon PS lamellar thickness is found. For the samples with lamellar morphology the hardness value was found to correlate with the mechanical parameters obtained by uni-axial tensile testing according to: H/sY approx. equal to 2.2 and E/H approx. equal to 22.