An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions

8 figures, 2 tables.-- Supplementary information available.

Detalhes bibliográficos
Autores: Zhou, Yingdong, Remón, Javier, Ding, Wei, Jiang, Zhicheng, Pinilla Ibarz, José Luis, Hu, Changwei, Suelves Laiglesia, Isabel
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2024
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositório:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/359879
Acesso em linha:http://hdl.handle.net/10261/359879
Access Level:Acceso aberto
Palavra-chave:Microalgae
Almond hulls
Hydrothermal treatment
Seawater
Biorefinery
Co-valorization
http://metadata.un.org/sdg/7
Ensure access to affordable, reliable, sustainable and modern energy for all
Ensure sustainable consumption and production patterns
microalgae
seawater
almonds
Chlorella vulgaris
id ES_8bdba3d77cb79ff1c769d5c2cb21e144
oai_identifier_str oai:digital.csic.es:10261/359879
network_acronym_str ES
network_name_str España
repository_id_str
dc.title.none.fl_str_mv An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
title An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
spellingShingle An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
Zhou, Yingdong
Microalgae
Almond hulls
Hydrothermal treatment
Seawater
Biorefinery
Co-valorization
http://metadata.un.org/sdg/7
Ensure access to affordable, reliable, sustainable and modern energy for all
Ensure sustainable consumption and production patterns
microalgae
seawater
almonds
Chlorella vulgaris
title_short An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
title_full An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
title_fullStr An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
title_full_unstemmed An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
title_sort An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions
dc.creator.none.fl_str_mv Zhou, Yingdong
Remón, Javier
Ding, Wei
Jiang, Zhicheng
Pinilla Ibarz, José Luis
Hu, Changwei
Suelves Laiglesia, Isabel
author Zhou, Yingdong
author_facet Zhou, Yingdong
Remón, Javier
Ding, Wei
Jiang, Zhicheng
Pinilla Ibarz, José Luis
Hu, Changwei
Suelves Laiglesia, Isabel
author_role author
author2 Remón, Javier
Ding, Wei
Jiang, Zhicheng
Pinilla Ibarz, José Luis
Hu, Changwei
Suelves Laiglesia, Isabel
author2_role author
author
author
author
author
author
dc.contributor.none.fl_str_mv Ministerio de Ciencia e Innovación (España)
Agencia Estatal de Investigación (España)
Gobierno de Aragón
National Natural Science Foundation of China
British Council
Beijing Municipal Natural Science Foundation
China Scholarship Council
European Commission
Zhou, Yingdong [0000-0003-0909-4704]
Remón, Javier [0000-0003-3315-5933]
Ding, Wei [0000-0002-6818-7524]
Jiang, Zhicheng [0000-0002-8096-4971]
Pinilla Ibarz, José Luis [0000-0002-8304-9656]
Hu, Changwei [0000-0002-4094-6605]
Suelves Laiglesia, Isabel [0000-0001-8437-2204]
Remón, Javier [jrn@unizar.es]
Hu, Changwei [changweihu@scu.edu.cn]
Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]
dc.subject.none.fl_str_mv Microalgae
Almond hulls
Hydrothermal treatment
Seawater
Biorefinery
Co-valorization
http://metadata.un.org/sdg/7
Ensure access to affordable, reliable, sustainable and modern energy for all
Ensure sustainable consumption and production patterns
microalgae
seawater
almonds
Chlorella vulgaris
topic Microalgae
Almond hulls
Hydrothermal treatment
Seawater
Biorefinery
Co-valorization
http://metadata.un.org/sdg/7
Ensure access to affordable, reliable, sustainable and modern energy for all
Ensure sustainable consumption and production patterns
microalgae
seawater
almonds
Chlorella vulgaris
description 8 figures, 2 tables.-- Supplementary information available.
publishDate 2024
dc.date.none.fl_str_mv 2024
2024
2024
dc.type.none.fl_str_mv info:eu-repo/semantics/article
http://purl.org/coar/resource_type/c_6501
Publisher's version
info:eu-repo/semantics/publishedVersion
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/10261/359879
url http://hdl.handle.net/10261/359879
dc.language.none.fl_str_mv Inglés
language_invalid_str_mv Inglés
dc.relation.none.fl_str_mv #PLACEHOLDER_PARENT_METADATA_VALUE#
info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-115053RB-I00
Zhou, Yingdong; Remón, Javier; Ding, Wei; Jiang, Zhicheng; Pinilla Ibarz, José Luis; Hu, Changwei; Suelves Laiglesia, Isabel; 2024; Supplementary data for An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions [Dataset]; Elsevier; http://dx.doi.org/10.1016/j.jclepro.2024.142719
http://dx.doi.org/10.1016/j.jclepro.2024.142719
Sí
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
eu_rights_str_mv openAccess
dc.format.none.fl_str_mv application/pdf
dc.publisher.none.fl_str_mv Elsevier
publisher.none.fl_str_mv Elsevier
dc.source.none.fl_str_mv reponame:DIGITAL.CSIC. Repositorio Institucional del CSIC
instname:Consejo Superior de Investigaciones Científicas (CSIC)
instname_str Consejo Superior de Investigaciones Científicas (CSIC)
reponame_str DIGITAL.CSIC. Repositorio Institucional del CSIC
collection DIGITAL.CSIC. Repositorio Institucional del CSIC
repository.name.fl_str_mv
repository.mail.fl_str_mv
_version_ 1869412856524439552
spelling An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditionsZhou, YingdongRemón, JavierDing, WeiJiang, ZhichengPinilla Ibarz, José LuisHu, ChangweiSuelves Laiglesia, IsabelMicroalgaeAlmond hullsHydrothermal treatmentSeawaterBiorefineryCo-valorizationhttp://metadata.un.org/sdg/7Ensure access to affordable, reliable, sustainable and modern energy for allEnsure sustainable consumption and production patternsmicroalgaeseawateralmondsChlorella vulgaris8 figures, 2 tables.-- Supplementary information available.This study explores the co-hydrothermal treatment (co-HTT) of almond hulls and Chlorella Vulgaris using seawater as an alternative HTT medium. The influence of the feedstock (individual biomass and all the possible binary mixtures) was systematically evaluated under different conditions (reaction temperatures and times). The feedstock mixture and hydrothermal conditions significantly influenced the overall product distribution: gas (1–5%), hydrochar (6–56%), biocrude (6–55%), and aqueous fraction (33–52%), along with the most representative physicochemical and fuel properties of these products. Notably, the biocrude had a calorific value of 24–31 MJ/kg, whereas the hydrochar shifted between 3 and 26 MJ/kg. The degradation of abundant polysaccharides in almond hulls produced acidic species, promoting the degradation of proteins to N-containing species in biocrude. The synergies between microalgae and almond hulls favored the deamination of amino acid and repolymerization of formed monomers. Process optimization revealed that the best biocrude production (59% yield and HHV = 28 MJ/kg) was obtained by treating C. Vulgaris at 268 °C for 180 min. Contrarily, the HTT of almond hulls under optimum processing conditions (300 °C and 112 min) also produced an energy-dense biocrude (29 MJ/kg) but with a much lesser yield (16%). However, such a low biocrude production can be synergistically increased up to 33 %, maintaining the HHV (31 MJ/kg), including up to 61 wt% of C.Vulgaris into the feedstock, with a feedstock energy recovery of 75%. Holistically, the co-HTT of 40 wt% C. Vulgaris and 60 wt% almond hulls at 300 °C for 180 min produced energy-dense liquid (23% yield and HHV = 32 MJ/kg) and solid (29% yield and HHV = 25 MJ/kg) biofuels simultaneously, with a feedstock energy recovery of 80%. Given these excellent prospects, this strategy provides timely and new insights into developing synergetic strategies to utilize microalgal and lignocellulosic biomasses more efficiently, paving the way toward developing holistic and unseasonal biorefinery processes.This work was funded by MCIN/AEI/10.13039/501100011033 (I + D + i project PID2020-115053RB-I00) and by the Aragón Government (Research Group Reference T06-23R). This work was also financially supported by the National Natural Science Foundation of China (No. 21536007), the 111 project (B17030), and the Beijing Nova Program (Z211100002121085). Yingdong Zhou acknowledges the support from the China Scholarship Council (CSC No. 202006240156). Javier Remón is grateful to the Spanish Ministry of Science, Innovation and Universities for the Juan de la Cierva (JdC) fellowship (Grant Number IJC2018-037110-I) and thanks MCIN/AEI/10.13039/501100011033 and the European Union « NextGenerationEU»/PRTR » for the Ramón y Cajal Fellowship (RYC2021-033368-I) awarded, and the Aragón Government (Research Group Reference T22_23R) for providing frame support.Peer reviewedElsevierMinisterio de Ciencia e Innovación (España)Agencia Estatal de Investigación (España)Gobierno de AragónNational Natural Science Foundation of ChinaBritish CouncilBeijing Municipal Natural Science FoundationChina Scholarship CouncilEuropean CommissionZhou, Yingdong [0000-0003-0909-4704]Remón, Javier [0000-0003-3315-5933]Ding, Wei [0000-0002-6818-7524]Jiang, Zhicheng [0000-0002-8096-4971]Pinilla Ibarz, José Luis [0000-0002-8304-9656]Hu, Changwei [0000-0002-4094-6605]Suelves Laiglesia, Isabel [0000-0001-8437-2204]Remón, Javier [jrn@unizar.es]Hu, Changwei [changweihu@scu.edu.cn]Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72]202420242024info:eu-repo/semantics/articlehttp://purl.org/coar/resource_type/c_6501Publisher's versioninfo:eu-repo/semantics/publishedVersionapplication/pdfhttp://hdl.handle.net/10261/359879reponame:DIGITAL.CSIC. Repositorio Institucional del CSICinstname:Consejo Superior de Investigaciones Científicas (CSIC)Inglés#PLACEHOLDER_PARENT_METADATA_VALUE#info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2020-115053RB-I00Zhou, Yingdong; Remón, Javier; Ding, Wei; Jiang, Zhicheng; Pinilla Ibarz, José Luis; Hu, Changwei; Suelves Laiglesia, Isabel; 2024; Supplementary data for An innovative ‘sea-thermal’ synergetic biorefinery for biofuel production: Co-valorization of lignocellulosic and algal biomasses using seawater under hydrothermal conditions [Dataset]; Elsevier; http://dx.doi.org/10.1016/j.jclepro.2024.142719http://dx.doi.org/10.1016/j.jclepro.2024.142719Síinfo:eu-repo/semantics/openAccessoai:digital.csic.es:10261/3598792026-05-22T06:33:51Z
score 15,812455

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