Electrostatic long-range stereocontrol in asymmetric Suzuki-Miyaura cross-coupling

In this issue of Chem Catalysis, Zhu and co-workers report on the development of asymmetric Suzuki-Miyaura cross-coupling using ligand-substrate electrostatic attractive interactions as the key strategy of stereocontrol. Using a sterically unbiased meta-carboxylate-substituted RuPhos derivative as t...

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Bibliographic Details
Author: Lassaletta, José M.
Format: article
Status:Versión enviada para evaluación y publicación
Publication Date:2023
Country:España
Institution:Consejo Superior de Investigaciones Científicas (CSIC)
Repository:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/354753
Online Access:http://hdl.handle.net/10261/354753
https://api.elsevier.com/content/abstract/scopus_id/85150337518
Access Level:Open access
Keyword:Electrostatic
Suzuki-Miyaura
long-range stereocontrol
asymmetric
Description
Summary:In this issue of Chem Catalysis, Zhu and co-workers report on the development of asymmetric Suzuki-Miyaura cross-coupling using ligand-substrate electrostatic attractive interactions as the key strategy of stereocontrol. Using a sterically unbiased meta-carboxylate-substituted RuPhos derivative as the ligand, they achieved high enantioselectivities not only in the coupling of substrates decorated with acidic, deprotonable functionalities at ortho-positions but also for meta-substituted analogs.