Magnetic carbon gate electrodes for the development of electrolyte-gated organic field effect transistor bio-sensing platforms
Electrolyte-gated organic field-effect transistors (EGOFETs) are promising devices for the development of bio-sensors. Typically, a gold gate electrode is functionalised with a self-assembled monolayer bearing the bio-receptor. Here, we propose a new route to fabricate EGOFET sensors using magnetic...
| Autores: | , , , |
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| Tipo de documento: | artigo |
| Estado: | Versão publicada |
| Data de publicação: | 2023 |
| País: | España |
| Recursos: | Consejo Superior de Investigaciones Científicas (CSIC) |
| Repositório: | DIGITAL.CSIC. Repositorio Institucional del CSIC |
| OAI Identifier: | oai:digital.csic.es:10261/340767 |
| Acesso em linha: | http://hdl.handle.net/10261/340767 https://api.elsevier.com/content/abstract/scopus_id/85169546163 |
| Access Level: | Acceso aberto |
| Palavra-chave: | Paste electrodes Biosensors Polymers |
| Resumo: | Electrolyte-gated organic field-effect transistors (EGOFETs) are promising devices for the development of bio-sensors. Typically, a gold gate electrode is functionalised with a self-assembled monolayer bearing the bio-receptor. Here, we propose a new route to fabricate EGOFET sensors using magnetic carbon-paste gate electrodes. In this way, magnetic nanoparticles properly modified with a bio-receptor are incubated with the analyte and, subsequently, collected on the gate electrode surface. Remarkably, these electrodes can be polished and re-used after each measurement. The feasibility of this route is here demonstrated for the biotin-avidin/streptavidin supramolecular complexes. High sensitivities and low limits of detection of the order of fM are achieved. Hence, this work demonstrates a novel and versatile strategy to exploit EGOFETs as sensing platforms. |
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