Probing Iceland's dust-emitting sediments: Particle size distribution, mineralogy, cohesion, Fe mode of occurrence, and reflectance spectra signatures

Characterising the physico-chemical properties of dust-emitting sediments in arid regions is fundamental to understanding the effects of dust on climate and ecosystems. However, knowledge regarding highlatitude dust (HLD) remains limited. This study focuses on analysing the particle size distributio...

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Detalles Bibliográficos
Autores: González-Romero, Adolfo, González-Flórez, Cristina, Panta, Agnesh, Yus-Díez, Jesús, Córdoba, Patricia, Alastuey, Andrés, Moreno, Natalia, Kandler, Konrad, Klose, Martina, Clark, Roger N., Ehlmann, Bethany L., Greenberger, Rebecca N., Keebler, Abigail M., Brodrick, Phil, Green, Robert O., Querol, Xavier, Pérez García-Pando, Carlos
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2024
País:España
Institución:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/361903
Acceso en línea:http://hdl.handle.net/10261/361903
https://api.elsevier.com/content/abstract/scopus_id/85196257982
Access Level:acceso abierto
Palabra clave:Dust
Pollution
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Descripción
Sumario:Characterising the physico-chemical properties of dust-emitting sediments in arid regions is fundamental to understanding the effects of dust on climate and ecosystems. However, knowledge regarding highlatitude dust (HLD) remains limited. This study focuses on analysing the particle size distribution (PSD), mineralogy, cohesion, iron (Fe) mode of occurrence, and visible-near infrared (VNIR) reflectance spectra of dustemitting sediments from dust hotspots in Iceland (HLD region). Extensive analysis was conducted on samples of top sediments, sediments, and aeolian ripples collected from seven dust sources, with particular emphasis on the Jökulsá basin, encompassing the desert of Dyngjunsandur. Both fully and minimally dispersed PSDs and their respective mass median particle diameters revealed remarkable similarities (56±69 and 55±62 μm, respectively). Mineralogical analyses indicated the prevalence of amorphous phases (68±26 %), feldspars (17±13 %), and pyroxenes (9.3±7.2 %), consistent with thorough analyses of VNIR reflectance spectra. The Fe content reached 9.5±0.40 wt %, predominantly within silicate structures (80±6.3 %), complemented by magnetite (16±5.5 %), hematite/goethite (4.5±2.7 %), and readily exchangeable Fe ions or Fe nano-oxides (1.6±0.63 %). Icelandic top sediments exhibited coarser PSDs compared to the high dust-emitting crusts from mid-latitude arid regions, distinctive mineralogy, and a 3-fold bulk Fe content, with a significant presence of magnetite. The congruence between fully and minimally dispersed PSDs underscores reduced particle aggregation and cohesion of Icelandic top sediments, suggesting that aerodynamic entrainment of dust could also play a role upon emission in this region, alongside saltation bombardment. The extensive analysis in Dyngjusandur enabled the development of a conceptual model to encapsulate Iceland's rapidly evolving high dust-emitting environments.