Germacranolides from Mikania guaco

Fourteen novel sesquiterpene lactones of the germacranolide type have been isolated from the aerial parts of Mikania guaco: six costunolide, two melampolide and six germacra-4-trans,10(14),11(13)-trien-12,6α-olide derivatives. Except for one compound all the others possess a carbonyl function at C-9...

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Detalhes bibliográficos
Autores: Rüngeler, Peter, Brecht, Volker, Tamayo Castillo, Giselle, Merfort, Irmgard
Tipo de documento: artigo
Data de publicação:2001
País:Costa Rica
Recursos:Universidad de Costa Rica
Repositório:Kérwá
Idioma:inglês
OAI Identifier:oai:kerwa.ucr.ac.cr:10669/87850
Acesso em linha:https://www.sciencedirect.com/science/article/pii/S0031942200003940#!
https://hdl.handle.net/10669/87850
Access Level:Acceso aberto
Palavra-chave:Mikania guaco
Asteraceae
Structure elucidation
Sesquiterpene lactones
Germacranolides
PHYTOCHEMISTRY
Descrição
Resumo:Fourteen novel sesquiterpene lactones of the germacranolide type have been isolated from the aerial parts of Mikania guaco: six costunolide, two melampolide and six germacra-4-trans,10(14),11(13)-trien-12,6α-olide derivatives. Except for one compound all the others possess a carbonyl function at C-9. Eight were obtained in the form of four isomer pairs which were difficult to separate. Structure elucidation was based on mass and 1D and 2D NMR measurements. Low energy conformations were obtained by quantum mechanical calculations. Pyrrolizidine alkaloids could not be detected.