Total Synthesis and Structural Validation of Phosdiecin A via Asymmetric Alcohol-Mediated Carbonyl Reductive Coupling

The first total synthesis and structural validation of phosdiecin A was accomplished in 13 steps through asymmetric iridium-catalyzed alcohol-mediated carbonyl reductive coupling. The present route is the shortest among >30 total and formal syntheses of fostriecin family members.

Detalhes bibliográficos
Autores: Della Felice, Franco, Sarotti, Ariel Marcelo, Krische, Michael J., Pilli, Ronaldo A.
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2019
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositório:CONICET Digital (CONICET)
Idioma:inglês
OAI Identifier:oai:ri.conicet.gov.ar:11336/117465
Acesso em linha:http://hdl.handle.net/11336/117465
Access Level:Acceso aberto
Palavra-chave:TOTAL SYNTHESIS
STRUCTURAL VALIDATION
PHOSDIECIN A
ASYMMETRIC CARBONYL REDUCTIVE COUPLING
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descrição
Resumo:The first total synthesis and structural validation of phosdiecin A was accomplished in 13 steps through asymmetric iridium-catalyzed alcohol-mediated carbonyl reductive coupling. The present route is the shortest among >30 total and formal syntheses of fostriecin family members.