Self-affine fractal electrodeposited gold surfaces : Characterization by scanning tunneling microscopy

The morphological evolution of columnar gold electrodeposits grown at 100 nm s <sup>−1</sup> by electroreducing a gold oxide layer on a gold cathode has been studied at a nanometer level by scanning tunneling microscopy. The interface thickness (ξ) depends on the scan length (L) as ξ∝ L...

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Detalhes bibliográficos
Autores: Vázquez, L., Salvarezza, Roberto Carlos, Ocón, P., Herrasti, P., Vara, J. M., Arvia, Alejandro Jorge
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:1994
País:Argentina
Recursos:Universidad Nacional de La Plata
Repositório:SEDICI (UNLP)
Idioma:inglês
OAI Identifier:oai:sedici.unlp.edu.ar:10915/85650
Acesso em linha:http://sedici.unlp.edu.ar/handle/10915/85650
Access Level:Acceso aberto
Palavra-chave:Ciencias Exactas
Química
Fractales
electrodeposits
electroreduction
Oro
scanning tunneling microscopy
Óxidos
Descrição
Resumo:The morphological evolution of columnar gold electrodeposits grown at 100 nm s <sup>−1</sup> by electroreducing a gold oxide layer on a gold cathode has been studied at a nanometer level by scanning tunneling microscopy. The interface thickness (ξ) depends on the scan length (L) as ξ∝ L <sup>α</sup> with α=0.49±0.07 for L > d<sub>s</sub>, where d<sub>s</sub> is the average top columnar size, and α=0.90±0.07 for L < d<sub>s</sub>. These results prove that the growing surface can be described as a self-affine fractal for length scales greater than the columnar size. Conversely, the columnar surface approaches the behavior of an Euclidean surface.