Surface modification of PVC membranes using fluorothiophenol compounds

The controlled chemical surface modification of PVC films by means of three fluoride aromatic compounds, 4-fluoro thiophenol, 3,4-difluorothiophenol and penta fluorothiophenol is reported. To obtain information about the surface selectivity of the reactions, the degree of modification of the polymer...

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Detalhes bibliográficos
Autores: Corrales, Marta, Bierbrauer, Karina Lilian, Sacristán, Hernán Javier, Mijangos, Carmen
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/187270
Acesso em linha:http://hdl.handle.net/11336/187270
Access Level:acceso abierto
Palavra-chave:AROMATIC FLUORINE COMPOUNDS
CONFOCAL RAMAN SPECTROSCOPY
POLY(VINYL CHLORIDE) (PVC)
SURFACE MODIFICATION
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descrição
Resumo:The controlled chemical surface modification of PVC films by means of three fluoride aromatic compounds, 4-fluoro thiophenol, 3,4-difluorothiophenol and penta fluorothiophenol is reported. To obtain information about the surface selectivity of the reactions, the degree of modification of the polymer across the film was determined by depth profiling carried out using confocal Raman microscopy. It is shown that the gradient of the modification degree and the surface selectivity depend on the relationship between the rate constants of the substitution reaction and the diffusion process of the reactant. Therefore it is function of reaction time, temperature and the proportion of solvent/nonsolvent used for the reaction.